大连理工大学侯军刚教授等人制备了多孔硫改性的镉结构,其具有良好的CO选择性。未改性的镉金属的低CO选择性表明了硫掺杂剂的引入实现了产物从HCOOH到CO的转变。机理研究表明,具有双协作位点的共价杂化sp带体系自然地打破了中间体结合能之间的线性相关性,从而实现了选择性调控。
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